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This article is based on documentation from Microsoft and has not been verified by the ThreatLocker team. 

Source: https://docs.microsoft.com/en-us/mem/intune/apps/intune-management-extension 

• Log into the ThreatLocker portal.
• Make sure you are managing the correct organization, or switch organizations using the Organizations page. 
• Click on the Computers page.
• Select Install New Computer. 

• Download the PowerShell Script for the group you are installing.

Add into Microsoft InTune.

Sign in to the Microsoft Endpoint Manager Admin Center.

• Select Devices > PowerShell scripts > Add. 

• Enter a script name and description and select Next. 

• Script Location: Browse to the location of your ThreatLockerPS1 Script and select Next.

• Select No under the "Enforce script signature check" section and select Next.

• Select No (default) runs the script in a 32-bit PowerShell host and select Next.
• Assign any Scope tags (Not required). 
• Select Groups, you wish to assign to.   

• Click next and Click Add to Add the Script.  

Please note: The endpoint will require a reboot in order for ThreatLocker to install.